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L27 · Lasers powered by scattering

Raman & Brillouin Lasers

Can transparent glass become a laser gain medium? Yes. A strong pump scatters off vibrations in the glass, molecular vibrations for Raman and sound waves for Brillouin, and amplifies light shifted to a lower frequency, called Stokes light. No population inversion is needed. Above threshold, the next Stokes order can grow, drain the previous one and hold it at a fixed level.

Pump a silica fiber past a Stokes threshold and watch the next order clamp the one before it. Capture a transient and calculate a steady pump sweep.

Interactive modelRaman & Brillouin Lasers
First Stokes steady noise-floor linewidth—\text{—}
Second Stokes steady noise-floor linewidth—\text{—}
Third Stokes steady noise-floor linewidth—\text{—}
Recorded phase-diffusion linewidth—\text{—}
Recorded phase samples—\text{—}
Scattering process—\text{—}
Elapsed round trips—\text{—}
Physical elapsed time—\text{—}
First Stokes frequency shift—\text{—}
First Stokes wavelength—\text{—}
Effective gain bandwidth—\text{—}
Feedback free spectral range—\text{—}
Gain overlap fraction—\text{—}
First oscillation threshold—\text{—}
Recorded pump in the fiber—\text{—}
First-order extracted power—\text{—}
Second-order extracted power—\text{—}
Third-order extracted power—\text{—}
Recorded phonon heat power—\text{—}
Recorded passive loss power—\text{—}
Recorded total Stokes output—\text{—}
Separate steady output reference—\text{—}
Integrated energy residual—\text{—}
Captured transient samples—\text{—}
Computed equilibrium samples—\text{—}
Frozen captured Stokes output—\text{—}
Stokes propagation—\text{—}
First-threshold regime—\text{—}

Physics tutorial

Scattered photons can sustain an oscillator

BackgroundThe pump light supplies the energy for both the Stokes light and the vibration it leaves in the material.

Why it mattersTransparent glass can still amplify light by scattering. Pump a silica fiber past a Stokes threshold, watch the next order clamp the one before it, then capture a transient and calculate a steady pump sweep.

Start with the essentials

Focus question
Can transparent glass become a laser gain medium?
One-sentence intuition
When the next Stokes order starts oscillating, it drains its parent and clamps it; it does not simply add more output.

Core mathematical model

One photon becomes light and vibration

νj−1=νj+Ωjhνj−1=hνj+hΩj\begin{aligned}\nu_{j-1}&=\nu_j+\Omega_j\\h\nu_{j-1}&=h\nu_j+h\Omega_j\end{aligned}

Each scattering event moves one photon from an order to the next, but the photons in the two orders carry different energies.

Average gain over the fiber

Cj=gjLeff/AeffLeff=(1−e−αL)/α\begin{aligned}C_j&=g_jL_{\rm eff}/A_{\rm eff}\\L_{\rm eff}&=(1-e^{-\alpha L})/\alpha\end{aligned}

The gain overlap includes the set error in mode spacing. A spectrally broad pump lowers the Brillouin gain.

Stokes growth and depletion

P˙j=Gj−DjGj=CjPj−1Pj−ΛPjDj=rjCj+1PjPj+1\begin{aligned}\dot P_j&=G_j-D_j\\G_j&=C_jP_{j-1}P_j-\Lambda P_j\\D_j&=r_jC_{j+1}P_jP_{j+1}\end{aligned}

Time here is counted in round trips. The frequency ratio in the depletion term accounts for the energy carried off by the emitted phonon.

First oscillation threshold

P0,th=Λ/C1Pin,th=aΛ/C1\begin{aligned}P_{0,\rm th}&=\Lambda/C_1\\P_{\rm in,th}&=a\Lambda/C_1\end{aligned}

The pump in the fiber decays with coefficient a. Each further Stokes order needs more power from its parent.

Heat left behind as phonons

Qph=∑j(rj−1−1)SjSj=CjPj−1Pjrj−1=νj−1/νj\begin{aligned}Q_{\rm ph}&=\sum_j(r_{j-1}-1)S_j\\S_j&=C_jP_{j-1}P_j\\r_{j-1}&=\nu_{j-1}/\nu_j\end{aligned}

The fraction of optical energy lost is small for Brillouin scattering and much larger for Raman scattering.

In steady state the parent is clamped

CjPj−1=Λ+rjCj+1Pj+1Pj>0\begin{aligned}C_jP_{j-1}&=\Lambda+r_jC_{j+1}P_{j+1}\\P_j&>0\end{aligned}

This relation gives every order that oscillates in a steady-state branch. The last order has no higher order to drain it.

Fundamental linewidth of each output

Nm=Pmtrt/(hνm)Am=γ(nˉ+1)Bm=2μmNm+1(2nˉ+1)Δνm=(Am+Bm)/(4πNm)\begin{aligned}N_m&=P_m t_{\rm rt}/(h\nu_m)\\A_m&=\gamma(\bar n+1)\\B_m&=2\mu_mN_{m+1}(2\bar n+1)\\\Delta\nu_m&=(A_m+B_m)/(4\pi N_m)\end{aligned}

A separate model of small phase fluctuations at low offset frequency uses the same steady powers. When the next order lases, it adds anti-Stokes noise. Technical noise from the pump is left out.

Record phase, then test coherence

dφ=2πΔνm dWg(1)(t)=e−πΔνm∣t∣Δν^=Var⁡(δφ)2πδt\begin{aligned}d\varphi&=\sqrt{2\pi\Delta\nu_m}\,dW\\g^{(1)}(t)&=e^{-\pi\Delta\nu_m|t|}\\\widehat{\Delta\nu}&=\frac{\operatorname{Var}(\delta\varphi)}{2\pi\delta t}\end{aligned}

The simulated phase record lets you check the diffusion and the coherence. The Fourier transform of the exponential coherence is a Lorentzian with this full width.

Common difficulties

The gain width is the output linewidth

Typical misconceptionThe gain bandwidth shown tells you the linewidth of the emitted laser light.

Better mental modelThe gain bandwidth belongs to the power model. The separate phase model calculates the steady, phase-matched noise floor and records how the phase diffuses. Technical pump noise and fluctuations near threshold are outside its scope.

More pump always grows the first order

Typical misconceptionEvery Stokes order keeps growing as the pump increases.

Better mental modelOnce the next order oscillates, it drains its parent, and the parent stays clamped on that branch.

Run the experiment

  1. 01

    Cross the threshold

    Compare Below threshold with Raman, then drag the pump dial. Each setting records six hundred round trips automatically.

    What to observe: The fixed seed light dies away below threshold and grows above it, until pump depletion limits the growth.
  2. 02

    Follow the energy into another order

    Choose Cascaded orders and follow the three colored outputs and the pump sweep below. Open Advanced controls to compare One allowed order.

    What to observe: As a new order grows, its parent is clamped. The separately calculated sweep shows the thresholds one after another.
  3. 03

    Broaden the pump

    Compare narrow and broad Brillouin pumping at the same power, and look at the backward and forward ports.

    What to observe: Less overlap raises the threshold. Odd and even Brillouin orders leave through opposite ports.
  4. 04

    Measure the output phase

    Open Advanced controls, choose One allowed order and click Record output phase. Expand the separate phase-noise record below, then compare it with a cascade.

    What to observe: The emitted linewidth is not the gain bandwidth, and in a cascade the next order adds its own noise channel.

Related experiments and articles

Probes and measurement · Reading path

Molecules, forces and ultrafast dynamics

Articles on this path that use this experiment, followed by the other experiments they suggest.

  1. ArticleRaman: the shifted lines moved with the source
  2. LabSpontaneous Raman SpectrometerMeasure a spontaneous Raman spectrum
  3. LabVibrational EELS: Resolution & Aloof ProbesCompare electron energy-loss spectroscopy
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