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FR26 · Elastic instability

Elastic Instability: Symmetry Breaking in a Four-Roll Mill

How can a slow polymer flow with no inertia at all lose its symmetry and start to oscillate? Through elastic stress alone. At the central stagnation point the flow stretches polymers into a thin, strongly stressed strand, and that stress pushes back on the flow. Above a Weissenberg number of about 5 a tiny tilt of the strand grows instead of fading, so the four rolls lose their symmetry. Near 10 the flow keeps oscillating and mixes fluid between the rolls, still with no inertia at all.

Four rolls stir a polymer solution with no inertia. Past a critical Weissenberg number, stretched polymers at the center break symmetry and the flow oscillates.

Interactive modelElastic Instability: Symmetry Breaking in a Four-Roll Mill
Stress asymmetry49.449.4
Flow at the probe−0.0282-0.0282
Mixing index of the tracers0.6460.646
Smallest stretch eigenvalue0.3260.326
Flow at the probe
Distance from symmetry
Where quadrant I’s dye came from
More numbers and how they are computed
Model time
00
Polymer coupling
00
Artificial stress diffusion
00
Grid and time step
00
Central stagnation point
00
Largest stretch, trace of the conformation tensor
00
Smallest stretch eigenvalue since this run started
00
Relative residual of the Stokes energy identity
00
Stress spectrum in the outer third of wavenumbers
00
Advective Courant number
00
Dye released at
00
Model time per wall-clock second
00

The asymmetry is the root-mean-square difference between the stress and its average over the symmetries of the roll force; it is zero for a symmetric state. The mixing index is one for dye spread evenly over the four quadrants and zero for dye still in its starting quadrant. A negative smallest eigenvalue means the stretch field is not physical there: the grid is too coarse for the stress strand. Every curve is computed by this simulation; none is measured data or a published curve.

Physics tutorial

Symmetry lost without inertia

BackgroundFour counter-rotating rolls stir a liquid so slowly that inertia plays no part. A plain liquid then follows the force exactly: the flow has the same symmetry as the stirring and never changes. Add long polymers and the same slow stirring can produce a flow that leans to one side and keeps oscillating.

Why it mattersAt the center of the four rolls is a stagnation point where the flow stretches polymers without limit. The stretched polymers form a thin strand of stress that pushes back on the flow. This is the simplest setting in which elastic stress alone breaks a symmetry, the first step toward elastic turbulence.

Start with the essentials

Focus question
How can a slow polymer flow with no inertia at all lose its symmetry and start to oscillate?
One-sentence intuition
The Weissenberg number Wi\mathrm{Wi} compares how long polymers remember a stretch with the flow time, in which the plain flow stretches the fluid at the center by a factor e. Once Wi\mathrm{Wi} passes about 4.9, the symmetric stress strand is unstable: a small tilt of the strand bends the flow so that it stretches the strand further in the same direction.

Core mathematical model

Slow flow driven by the rolls and the polymers

−Δu+∇p=β ∇⋅S+f,∇⋅u=0-\Delta\mathbf u+\nabla p=\beta\,\nabla\cdot\mathbf S+\mathbf f,\qquad \nabla\cdot\mathbf u=0

Stokes flow: viscosity balances the fixed roll force f\mathbf f and the polymer stress. With S=I\mathbf S=\mathbf I the flow is four symmetric cells around a central stagnation point.

How the polymers stretch and relax

∂tS+u⋅∇S−∇u S−S ∇uT=−S−IWi+νpΔS\partial_t\mathbf S+\mathbf u\cdot\nabla\mathbf S-\nabla\mathbf u\,\mathbf S-\mathbf S\,\nabla\mathbf u^{\mathsf T}=-\frac{\mathbf S-\mathbf I}{\mathrm{Wi}}+\nu_p\Delta\mathbf S

The Oldroyd-B conformation tensor S\mathbf S is carried and stretched by the flow and relaxes back to I\mathbf I. The small diffusion νp\nu_p is a numerical device the published runs also use; it is not a property of real polymers.

Stretching at the stagnation point

dSxxdt=2ε˙ Sxx−Sxx−1Wi,ε˙ Wi>12 ⇒ Sxx grows exponentially\frac{d S_{xx}}{dt}=2\dot\varepsilon\, S_{xx}-\frac{S_{xx}-1}{\mathrm{Wi}},\qquad \dot\varepsilon\,\mathrm{Wi}>\tfrac12\ \Rightarrow\ S_{xx}\ \text{grows exponentially}

ε˙\dot\varepsilon is the strain rate at the center in flow-time units: 1 for the solvent alone, and lower once the polymers resist, 2/32/3 in the limit of small Wi\mathrm{Wi}. Past ε˙ Wi=1/2\dot\varepsilon\,\mathrm{Wi}=1/2 stretching outruns relaxation; without diffusion the central stress then grows without bound, from Wi≈0.9\mathrm{Wi}\approx0.9 in Thomases and Shelley (2007). Here diffusion and the feedback on the flow keep the strand finite.

Measuring the lost symmetry

A=⟨∥Q−PQ∥F2⟩1/2,Q=S−IA=\left\langle\left\|\mathbf Q-\mathcal P\mathbf Q\right\|_F^2\right\rangle^{1/2},\qquad \mathbf Q=\mathbf S-\mathbf I

P\mathcal P averages the stress over the symmetries of the roll force. AA is zero for a symmetric state and grows exponentially once the symmetric strand is unstable.

Common difficulties

Instability needs inertia?

Typical misconceptionA flow this slow cannot become unstable; instabilities and turbulence need a large Reynolds number.

Better mental modelHere the Reynolds number is zero by construction. The nonlinearity that drives the instability is in the polymer equation: the flow stretches the polymers and the stretched polymers bend the flow.

The numbers are converged

Typical misconceptionThe threshold and periods shown here are the exact answer of the model.

Better mental modelThe threshold 4.86 agrees between our 64 by 64 and 128 by 128 grids and with the published 4.8 to 4.9. At the default grid the smallest eigenvalue of S\mathbf S briefly turns negative while the strand forms, so that stage is under-resolved. Changing νp\nu_p changes the long-time behavior.

Run the experiment

  1. 01

    Watch the oscillation

    Start with Oscillation that mixes and follow the probe chart and the colored dye.

    What to observe: The bright stress strand sways off center, the probe velocity swings with a long and a short period, and dye from quadrants II and IV keeps entering quadrant I, while little arrives from the opposite quadrant III.
  2. 02

    Stay below the threshold

    Choose Symmetric stress strand, then drag the Weissenberg slider from 4 up past 5.

    What to observe: At 4 the strand stays straight and the asymmetry decays. Above about 4.9 it starts to rise instead; at 6 it climbs as a straight line on the log axis and the strand tips over after a few hundred flow times.
  3. 03

    Smear the stress

    Choose Too much stress diffusion and compare it with the reference oscillation.

    What to observe: Ten times the published diffusion delays the symmetry breaking to about 590 flow times and leaves only a weak slow wobble.

Related experiments and articles

Complex fluids · Reading path

Relaxation, stretching, extension and elastic instability

Articles on this path that use this experiment, followed by the other experiments they suggest.

  1. ArticleHow normal stress along curved streamlines drives elastic instability
  2. LabCoil–Stretch Transition: Polymers in Shear and ExtensionRead the ratio of normal stress to shear stress
  3. ArticleHow a four-roll flow loses symmetry at its stagnation point, and how much the numerics change it
  4. ArticleReading elastic turbulence: the evidence for chaotic flow without inertia, and what is still open
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